应该填whose (C.D)
窗子是蓝色的那栋楼房是我们的校图书馆.
这是一个定语从句,先行词是the building,
这个定语从句的引导词/连接词whose在从句中作定语,修饰the windows,表示这栋大楼的（窗子）.
而关系代词which和that都不能作定语.
希望我的解释能让你明白.
the building ___the windows are biue is our schooi library
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